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H-aggregate has the cofacial, parallel molecular stacking with slip angle larger than 54.7° (Figure 1). In H-aggregates, the molecular transition dipoles are oriented "side-by-side," in which the lower excited state of the two split energy levels generated by dipole interactions is optically forbidden, while the higher one is allowed.

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The more frequently used term, "topology," focuses on the connectivity of networks of MOFs [ 41, 42] while phase emphasizes the packing mode of metal ions/nodes and linkers. To align with the terminology of PEN, in this review, we adopt "phase" to describe the ordered arrangements of metal nodes and linkers of MOFs.